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© Stefan Marzenell

Z-Scan

To understand the effects which influence the pulse formation in the AgGaSe2-OPO, i.e. the pulse duration and pulse chirp of signal and idler pulses, a numerical simulation is in progress, at present. For the calculation of self and cross phase modulation the nonlinear refractive index of AgGaSe2 was measured using the Z-Scan method.

First the well known Z-Scan technique with an aperture and a detector was used to determine the nonlinear index of refraction.

With the known numbers of wavelength, beam waist, power, repetition rate and pulse duration the nonlinear index of refraction was determined to be

      g = ( 6.35 +/- 0.70 ) 10-18 m2/W or

      n2 = ( 4.00 +/- 0.45 ) 10-11 esu.

Second a new technique with an ir camera was used. The beam structure in the far field was measured using this camera while the AgGaSe2 crystal was moved through the beam waist. A few examples of these measurements are shown below.

From these measurements the maximum transmission and the integrated transmission are deduced. For a (nonlinear) absorption measurement the data of the integrated transmission are normalized. We found at  a wavelength of 1.58 µm no nonlinear absorption. For the Z-Scan measurement the data of the maximum transmission are normalized. These data are shown below.

Again with the known numbers of wavelength, beam waist, power, repetition rate and pulse duration the nonlinear index of refraction was determined to be

      g = ( 6.07 +/- 1.05 ) 10-18 m2/W or

      n2 = ( 3.81 +/- 0.65 ) 10-11 esu.

Using these numbers of the nonlinear index of refraction the numerical prediction of pulse duration and pulse chirp shows good agreement with the measured values.

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